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Ac hopping conduction at extreme disorder takes place on the percolating cluster
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Ac hopping conduction at extreme disorder takes place on the percolating cluster
Thomas B. Schr?der and Jeppe C. Dyre
DNRF Centre “Glass and Time,” IMFUFA, Department of Sciences,
Roskilde University, Postbox 260, DK-4000 Roskilde, Denmark
(Dated: June 6, 2008)
Simulations of the random barrier model show that ac currents at extreme disorder are carried
almost entirely by the percolating cluster slightly above threshold; thus contributions from isolated
low-activation-energy clusters are negligible. The effective medium approximation in conjunction
with the Alexander-Orbach conjecture leads to an excellent analytical fit to the universal ac con-
ductivity with no nontrivial fitting parameters.
Recent advances relating to ion conduction in glasses
and other disordered solids include the application of
multidimensional NMR techniques [1], the introduction
of ac nonlinear spectroscopy [2], and elucidations of the
high-frequency nearly constant loss [3]. Moreover, it was
found that the old idea of ions moving by the vacancy
mechanism may well be correct [4], and simulations gave
new insight into the mixed-alkali effect [5]. Despite these
and other significant advances, important questions re-
main unanswered. For instance, it is still not understood
what role is played by ion interactions for the conductiv-
ity [6], or why the random barrier model (RBM) [7, 8]
represents ac conductivity data so well. The latter ques-
tion is not answered below, but new simulations and ar-
guments are presented that we believe lead to a full un-
derstanding of the physics of the RBM in the extreme
disorder limit (low temperature limit).
Ac conductivity is often studied also for amorphous
semiconductors, electronically or ionically conducting
polymers, defective crystals of various kinds, polaronic
conductors, etc [7, 8]. It is a longstanding observation
that all disordered solids have remarkably sim
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