metal-catalyzed α-arylation of carbonyl and related molecules novel trends in c xf8ff;c bond formation by c xf8ff;h bond functionalization文档.pdfVIP
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metal-catalyzed α-arylation of carbonyl and related molecules novel trends in c xf8ff;c bond formation by c xf8ff;h bond functionalization文档
Reviews T. J. Colacot and C. C. C. Johansson
DOI: 10.1002/anie.200903424
a-Arylation
Metal-Catalyzed a-Arylation of Carbonyl and Related
Molecules: Novel Trends in CC Bond Formation by
C H Bond Functionalization
Carin C. C. Johansson and Thomas J. Colacot*
Keywords:
a-arylation · CC coupling ·
carbonyl compounds ·
homogeneous catalysis
Angewandte
Chemie
676 2010 Wiley-VCH Verlag GmbH Co. KGaA, Weinheim Angew. Chem. Int. Ed. 2010, 49, 676 – 707
Angewandte
a-Arylation Chemie
a-Arylated carbonyl compounds are commonly occurring motifs From the Contents
in biologically interesting molecules and are therefore of high
1. Introduction 677
interest to the pharmaceutical industry. Conventional procedures for
their synthesis often result in complications in scale-up, such as the 2. a-Arylation of Ketones 678
use of stoichiometric amounts of toxic reagents and harsh reaction
conditions. Over the last decade, significant efforts have been 3. Palladium-Catalyzed a-Arylation
directed towards the development of metal-catalyzed a-arylations of of Esters 687
carbonyl compounds as an alternative synthetic approach that
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